Part:BBa_K5152004
PbrR-pPbr lead sensing chromoprotein reporter device
Our biosensor construct for detecting heavy metal lead is inspired by iGEM 2007 Team Brown (BBa_I721001). The regulatory protein PbrR controls the pPbr promoter. When lead is present, PbrR forms a dimer, activating the expression of downstream coding sequences.
We employed this construct in E. coli, which doesn't naturally express PbrR, so we co-expressed it. We used dTomato as the reporter gene, an RFP with chromoprotein properties, chosen for its visible colour to avoid the need for expensive equipment. This sequence, optimized by our 2023 team, ensures vibrant and stable expression.
Our project examined the expression profiles of several chromoproteins, including amilCP, cjBlue, tsPurple, eforRed, and dTomato. For more details, please refer to our wiki page.
Usage and Biology
Lead Detection Functional Assay
Our biosensor effectively detected lead. After adding a final concentration of 100 µM lead (II) nitrate to the culture, cells exhibited visible red colouration in the pellet after 12 hours and significant culture colouration after 24 hours. We noted leaky expression with incubation times over 18 hours, suggesting a need to adjust the regulatory protein expression strength or incubation conditions.
Concentration Dependent Signals
We tested the biosensors with varying lead concentrations (0.01 µM to 1000 µM). After 24 hours, colo山r intensity was proportional to lead concentration, except at 500 µM and 1000 µM, likely due to toxicity affecting protein expression, as smaller pellet sizes were observed.
Reference
Borremans B, Hobman JL, Provoost A, Brown NL, van Der Lelie D. (2001) Cloning and functional analysis of the pbr lead resistance determinant of Ralstonia metallidurans CH34. J Bacteriol. 2001 Oct;183(19):5651-8. doi: 10.1128/JB.183.19.5651-5658.2001. PMID: 11544228; PMCID: PMC95457.
Wei W, Liu X, Sun P, Wang X, Zhu H, Hong M, Mao ZW, Zhao J. (2014) Simple whole-cell biodetection and bioremediation of heavy metals based on an engineered lead-specific operon. Environ Sci Technol. 2014 Mar 18;48(6):3363-71. doi: 10.1021/es4046567. Epub 2014 Mar 3. PMID: 24564581.
Chen P, Greenberg B, Taghavi S, Romano C, van der Lelie D, He C. (2005) An exceptionally selective lead(II)-regulatory protein from Ralstonia metallidurans: development of a fluorescent lead(II) probe. Angew Chem Int Ed Engl. 2005 Apr 29;44(18):2715-2719. doi: 10.1002/anie.200462443. PMID: 15800869.
Sequence and Features
- 10COMPATIBLE WITH RFC[10]
- 12INCOMPATIBLE WITH RFC[12]Illegal NheI site found at 35
Illegal NheI site found at 58 - 21COMPATIBLE WITH RFC[21]
- 23COMPATIBLE WITH RFC[23]
- 25COMPATIBLE WITH RFC[25]
- 1000INCOMPATIBLE WITH RFC[1000]Illegal SapI.rc site found at 714
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